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RSS FeedsIJERPH, Vol. 16, Pages 1439: Preparation and Characterization of Cu-Mn-Ce@?-Al2O3 to Catalyze Ozonation in Coal Chemical Wastewater-Biotreated Effluent (International Journal of Environmental Research and Public Health)

 
 

23 april 2019 12:02:14

 
IJERPH, Vol. 16, Pages 1439: Preparation and Characterization of Cu-Mn-Ce@?-Al2O3 to Catalyze Ozonation in Coal Chemical Wastewater-Biotreated Effluent (International Journal of Environmental Research and Public Health)
 


Cu-Mn-Ce@γ-Al2O3 was prepared by incipient wetness impregnation and used to catalyze ozonation in a coal chemical wastewater-biotreated effluent. The preparation factors that considerably affected the catalytic performance of Cu-Mn-Ce@γ-Al2O3, specifically metal oxide loading percentage, calcination temperature, and calcination time, were examined. The catalyst was characterized by scanning electron microscopy, energy dispersive spectrometry, X-ray diffraction, and Brunauer-Emmett-Teller analysis. The optimal catalytic ozonation operating parameters, such as ozone dosage, catalyst dosage, pH, and reaction time, were also investigated. Results showed that an optimized catalyst consisted of 17.0% CuO, 3.0% MnO2, and 2.0% CeO2 (wt.%). The optimal calcination temperature and calcination time were 600 °C and 5 h. The optimal catalytic ozonation operating parameters, including ozone dosage, catalyst dosage, pH, and reaction time, were 7, 80.0 mg/L, 20.0 mg/L, 7 and 50 min, respectively. The COD removal of biotreated effluent increased to 61% under these optimal operating conditions. Meanwhile, ozonation alone resulted in only 20% removal. This work proposes the use of easily available Cu-Mn-Ce@γ-Al2O3 catalyst and might drive the advancement of catalytic ozonation for chemical wastewater purification.


 
67 viewsCategory: Medicine, Pathology, Toxicology
 
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IJERPH, Vol. 16, Pages 1438: Residue Levels of Organochlorine Pesticides in Breast Milk and Its Associations with Cord Blood Thyroid Hormones and the Offspring`s Neurodevelopment (International Journal of Environmental Research and Public Health)
 
 
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